The production and processing of GRMs in the liquid phase, coupled with the ability to “on-demand” tune their optoelectronic properties exploiting wet-chemical functionalization, enable their effective integration in advanced PV devices through scalable, reliable, and inexpensive printing/coating processes. These components include front (transparent) and back conductive electrodes, charge transporting layers, and interconnecting/recombination layers, as well as photoactive layers. The mechanical, thermal, and optoelectronic properties of GRMs can be exploited in different active components of solar cells to design next-generation devices. In this context, graphene and related two-dimensional (2D) materials (GRMs), including nonlayered 2D materials and 2D perovskites, as well as their hybrid systems, are emerging as promising candidates to drive innovation in PV technologies. In the ever-increasing energy demand scenario, the development of novel photovoltaic (PV) technologies is considered to be one of the key solutions to fulfil the energy request. – Laboratory for Advanced Solar Energy, National University of Science and Technology “MISiS”, 119049 Leninskiy Prosect 6, Moscow, Russia g Department of Electrical & Computer Engineering, Hellenic Mediterranean University, Estavromenos 71410 Heraklion, Crete, Greece Stagno D’alcontres 37, 98158 Messina, Italy d CHOSE – Centre for Hybrid and Organic Solar Energy, University of Rome “Tor Vergata”, via del Politecnico 1, 00133 Roma, Italy e University of Pavia and INSTM, Via Taramelli 16, 27100 Pavia, Italy f L.A.S.E. E-mail: b Istituto Italiano di Tecnologia, Graphene Labs, via Moreogo 30, 16163 Genova, Italy c CNR-IPCF, Istituto per i Processi Chimico-Fisici, Via F. * ab a BeDimensional S.p.A., Via Lungotorrente Secca 30R, 16163 Genova, Italy. Rev., 2021, 50, 11870-11965 Solution-processed two-dimensional materials for next-generation photovoltaics
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